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John B. Asbury - Publications

Affiliations: 
Chemistry Pennsylvania State University, State College, PA, United States 
Area:
Organic photovoltaics, Quantum dots
Website:
http://www.chem.psu.edu/directory/jba11
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77 high-probability publications. We are testing a new system for linking publications to authors. You can help! If you notice any inaccuracies, please sign in and mark papers as correct or incorrect matches. If you identify any major omissions or other inaccuracies in the publication list, please let us know.

Year Citation  Score
2022 Pensack RD, Purdum GE, Mazza SM, Grieco C, Asbury JB, Anthony JE, Loo YL, Scholes GD. Excited-State Dynamics of 5,14- vs 6,13-Bis(trialkylsilylethynyl)-Substituted Pentacenes: Implications for Singlet Fission. The Journal of Physical Chemistry. C, Nanomaterials and Interfaces. 126: 9784-9793. PMID 35756579 DOI: 10.1021/acs.jpcc.2c00897  0.798
2021 Kennehan ER, Munson KT, Grieco C, Doucette GS, Marshall AR, Beard MC, Asbury JB. Influence of Ligand Structure on Excited State Surface Chemistry of Lead Sulfide Quantum Dots. Journal of the American Chemical Society. 143: 13824-13834. PMID 34420309 DOI: 10.1021/jacs.1c06248  0.721
2019 Grieco C, Doucette GS, Munson KT, Swartzfager JR, Munro JM, Anthony JE, Dabo I, Asbury JB. Vibrational probe of the origin of singlet exciton fission in TIPS-pentacene solutions. The Journal of Chemical Physics. 151: 154701. PMID 31640354 DOI: 10.1063/1.5116586  0.718
2019 Munson KT, Doucette GS, Kennehan ER, Swartzfager JR, Asbury JB. Vibrational Probe of the Structural Origins of Slow Recombination in Halide Perovskites The Journal of Physical Chemistry C. 123: 7061-7073. DOI: 10.1021/Acs.Jpcc.9B00555  0.423
2018 Aplan MP, Munro J, Lee Y, Brigeman AN, Grieco C, Wang Q, Giebink NC, Dabo I, Asbury JB, Gomez ED. Revealing the Importance of Energetic and Entropic Contributions to the Driving Force for Charge Photogeneration. Acs Applied Materials & Interfaces. PMID 30360072 DOI: 10.1021/Acsami.8B12077  0.747
2018 Pensack RD, Tilley AJ, Grieco C, Purdum GE, Ostroumov EE, Granger DB, Oblinsky DG, Dean JC, Doucette GS, Asbury JB, Loo YL, Seferos DS, Anthony JE, Scholes GD. Striking the right balance of intermolecular coupling for high-efficiency singlet fission. Chemical Science. 9: 6240-6259. PMID 30090312 DOI: 10.1039/C8Sc00293B  0.783
2018 Kennehan ER, Doucette GS, Marshall AR, Grieco C, Munson KT, Beard MC, Asbury JB. Electron-Phonon Coupling and Resonant Relaxation from 1D and 1P States in PbS Quantum Dots. Acs Nano. PMID 29792675 DOI: 10.1021/Acsnano.8B03216  0.697
2018 Grieco C, Kennehan ER, Kim H, Pensack RD, Brigeman AN, Rimshaw A, Payne MM, Anthony JE, Giebink NC, Scholes GD, Asbury JB. Direct Observation of Correlated Triplet Pair Dynamics during Singlet Fission Using Ultrafast Mid-IR Spectroscopy The Journal of Physical Chemistry C. 122: 2012-2022. DOI: 10.1021/Acs.Jpcc.7B11228  0.812
2018 Aplan MP, Grieco C, Lee Y, Munro JM, Lee W, Gray JL, Seibers ZD, Kuei B, Litofsky JH, Kilbey SM, Wang Q, Dabo I, Asbury JB, Gomez ED. Conjugated Block Copolymers as Model Systems to Examine Mechanisms of Charge Generation in Donor-Acceptor Materials Advanced Functional Materials. 29: 1804858. DOI: 10.1002/Adfm.201804858  0.693
2017 Grieco C, Kennehan E, Rimshaw AD, Payne MM, Anthony JE, Asbury JB. Harnessing Molecular Vibrations to Probe Triplet Dynamics During Singlet Fission. The Journal of Physical Chemistry Letters. PMID 29112418 DOI: 10.1021/Acs.Jpclett.7B02434  0.764
2017 Kennehan ER, Grieco C, Brigeman AN, Doucette GS, Rimshaw A, Bisgaier K, Giebink NC, Asbury JB. Using molecular vibrations to probe exciton delocalization in films of perylene diimides with ultrafast mid-IR spectroscopy. Physical Chemistry Chemical Physics : Pccp. PMID 28868536 DOI: 10.1039/C7Cp04819J  0.747
2017 Grieco C, Hirsekorn KF, Heitsch AT, Thomas AC, McAdon MH, Vanchura BA, Romanelli MM, Brehm LL, Leugers A, Sokolov A, Asbury JB. Mechanisms of Energy Transfer and Enhanced Stability of Carbidonitride Phosphors for Solid State Lighting. Acs Applied Materials & Interfaces. PMID 28319374 DOI: 10.1021/Acsami.6B15323  0.68
2017 Pensack RD, Grieco C, Purdum GE, Mazza SM, Tilley AJ, Ostroumov EE, Seferos DS, Loo Y, Asbury JB, Anthony JE, Scholes GD. Solution-processable, crystalline material for quantitative singlet fission Materials Horizons. 4: 915-923. DOI: 10.1039/C7Mh00303J  0.753
2017 Munson KT, Grieco C, Kennehan ER, Stewart RJ, Asbury JB. Time-Resolved Infrared Spectroscopy Directly Probes Free and Trapped Carriers in Organo-Halide Perovskites Acs Energy Letters. 2: 651-658. DOI: 10.1021/Acsenergylett.7B00033  0.737
2017 Grieco C, Doucette GS, Munro JM, Kennehan ER, Lee Y, Rimshaw A, Payne MM, Wonderling N, Anthony JE, Dabo I, Gomez ED, Asbury JB. Triplet Transfer Mediates Triplet Pair Separation during Singlet Fission in 6,13-Bis(triisopropylsilylethynyl)-Pentacene Advanced Functional Materials. 27: 1703929. DOI: 10.1002/Adfm.201703929  0.729
2016 Grieco C, Doucette GS, Pensack RD, Payne MM, Rimshaw A, Scholes GD, Anthony JE, Asbury JB. Dynamic Exchange During Triplet Transport in Nanocrystalline TIPS-Pentacene Films. Journal of the American Chemical Society. 138: 16069-16080. PMID 27960344 DOI: 10.1021/Jacs.6B10010  0.785
2016 Rimshaw A, Grieco C, Asbury JB. High Sensitivity Nanosecond Mid-Infrared Transient Absorption Spectrometer Enabling Low Excitation Density Measurements of Electronic Materials. Applied Spectroscopy. PMID 27324422 DOI: 10.1177/0003702816645606  0.724
2016 Pensack RD, Ostroumov EE, Tilley AJ, Mazza S, Grieco C, Thorley KJ, Asbury JB, Seferos DS, Anthony JE, Scholes GD. Observation of Two Triplet Pair Intermediates in Singlet Exciton Fission. The Journal of Physical Chemistry Letters. PMID 27281713 DOI: 10.1021/Acs.Jpclett.6B00947  0.8
2016 Stewart RJ, Grieco C, Larsen AV, Maier JJ, Asbury JB. Approaching Bulk Carrier Dynamics in Organo-Halide Perovskite Nanocrystalline Films by Surface Passivation. The Journal of Physical Chemistry Letters. 1148-1153. PMID 26966792 DOI: 10.1021/Acs.Jpclett.6B00366  0.712
2016 Stewart RJ, Grieco C, Larsen AV, Doucette GS, Asbury JB. Molecular Origins of Defects in Organohalide Perovskites and Their Influence on Charge Carrier Dynamics The Journal of Physical Chemistry C. 120: 12392-12402. DOI: 10.1021/Acs.Jpcc.6B03472  0.737
2016 Grieco C, Aplan MP, Rimshaw A, Lee Y, Le TP, Zhang W, Wang Q, Milner ST, Gomez ED, Asbury JB. Molecular Rectification in Conjugated Block Copolymer Photovoltaics Journal of Physical Chemistry C. 120: 6978-6988. DOI: 10.1021/Acs.Jpcc.6B00103  0.742
2015 Rimshaw A, Grieco C, Asbury JB. Note: Using fast digitizer acquisition and flexible resolution to enhance noise cancellation for high performance nanosecond transient absorbance spectroscopy. The Review of Scientific Instruments. 86: 066107. PMID 26133882 DOI: 10.1063/1.4923093  0.663
2015 Smith BH, Clark MB, Kuang H, Grieco C, Larsen AV, Zhu C, Wang C, Hexemer A, Asbury JB, Janik MJ, Gomez ED. Controlling Polymorphism in Poly(3-Hexylthiophene) through Addition of Ferrocene for Enhanced Charge Mobilities in Thin-Film Transistors Advanced Functional Materials. DOI: 10.1002/Adfm.201403089  0.716
2013 Liu X, Jeong KS, Williams BP, Vakhshouri K, Guo C, Han K, Gomez ED, Wang Q, Asbury JB. Tuning the dielectric properties of organic semiconductors via salt doping. The Journal of Physical Chemistry. B. 117: 15866-74. PMID 24073822 DOI: 10.1021/Jp408537P  0.669
2013 Jeong KS, Pensack RD, Asbury JB. Vibrational spectroscopy of electronic processes in emerging photovoltaic materials. Accounts of Chemical Research. 46: 1538-47. PMID 23514085 DOI: 10.1021/Ar300300M  0.812
2012 Jeong KS, Tang J, Liu H, Kim J, Schaefer AW, Kemp K, Levina L, Wang X, Hoogland S, Debnath R, Brzozowski L, Sargent EH, Asbury JB. Enhanced mobility-lifetime products in PbS colloidal quantum dot photovoltaics. Acs Nano. 6: 89-99. PMID 22168594 DOI: 10.1021/Nn2039164  0.625
2012 Pensack RD, Guo C, Vakhshouri K, Gomez ED, Asbury JB. Influence of acceptor structure on barriers to charge separation in organic photovoltaic materials Journal of Physical Chemistry C. 116: 4824-4831. DOI: 10.1021/Jp2083133  0.675
2011 Tang J, Kemp KW, Hoogland S, Jeong KS, Liu H, Levina L, Furukawa M, Wang X, Debnath R, Cha D, Chou KW, Fischer A, Amassian A, Asbury JB, Sargent EH. Colloidal-quantum-dot photovoltaics using atomic-ligand passivation. Nature Materials. 10: 765-71. PMID 21927006 DOI: 10.1038/Nmat3118  0.615
2011 Pensack RD, Asbury JB. Ultrafast probes of charge transfer states in organic photovoltaic materials Chemical Physics Letters. 515: 197-205. DOI: 10.1016/J.Cplett.2011.07.002  0.708
2010 Pensack RD, Banyas KM, Asbury JB. Vibrational solvatochromism in organic photovoltaic materials: method to distinguish molecules at donor/acceptor interfaces. Physical Chemistry Chemical Physics : Pccp. 12: 14144-52. PMID 20871905 DOI: 10.1039/C0Cp00971G  0.68
2010 Pensack RD, Banyas KM, Asbury JB. Temperature-independent vibrational dynamics in an organic photovoltaic material. The Journal of Physical Chemistry. B. 114: 12242-51. PMID 20812710 DOI: 10.1021/Jp105772Y  0.704
2010 Pensack RD, Banyas KM, Asbury JB. Vibrational energy nediates charge separation in organic photovoltaic materials Ieee Journal On Selected Topics in Quantum Electronics. 16: 1776-1783. DOI: 10.1109/Jstqe.2010.2041751  0.718
2010 Pensack RD, Asbury JB. Beyond the adiabatic limit: Charge photogeneration in organic photovoltaic materials Journal of Physical Chemistry Letters. 1: 2255-2263. DOI: 10.1021/Jz1005225  0.704
2010 Pensack RD, Banyas KM, Asbury JB. Charge trapping in organic photovoltaic materials examined with time-resolved vibrational spectroscopy Journal of Physical Chemistry C. 114: 5344-5350. DOI: 10.1021/Jp905061Y  0.727
2010 Pensack RD, Banyas KM, Asbury JB. Ultrafast IR spectroscopic study of free carrier formation in OPV polymer blends Acs Symposium Series. 1034: 53-69. DOI: 10.1021/bk-2010-1034.ch005  0.623
2010 Pensack RD, Banyas KM, Asbury JB. Charge separation in organic photovoltaic materials mediated by excess vibrational energy Acs National Meeting Book of Abstracts.  0.674
2009 Pensack RD, Asbury JB. Barrierless free carrier formation in an organic photovoltaic material measured with ultrafast vibrational spectroscopy. Journal of the American Chemical Society. 131: 15986-7. PMID 19886692 DOI: 10.1021/Ja906293Q  0.707
2009 Pensack RD, Banyas KM, Barbour LW, Hegadorn M, Asbury JB. Ultrafast vibrational spectroscopy of charge-carrier dynamics in organic photovoltaic materials. Physical Chemistry Chemical Physics : Pccp. 11: 2575-91. PMID 19421513 DOI: 10.1039/B817113K  0.734
2009 Pensack RD, Barbour LW, Hegadorn M, Asbury JB. Non-thermal free carrier formation in organic photovoltaic polymer blends Proceedings of Spie - the International Society For Optical Engineering. 7396. DOI: 10.1117/12.826373  0.707
2009 Pensack RD, Banyas KM, Asbury JB. Ultrafast IR spectroscopic study of free carrier formation and charge trapping in organic photovoltaic polymer blends Acs National Meeting Book of Abstracts.  0.655
2008 Pensack RD, Banyas KM, Barbour LW, Asbury JB. Interfacial charge separation and trapping in a photovoltaic polymer blend observed with ultrafast vibrational spectroscopy Proceedings of Spie - the International Society For Optical Engineering. 7034. DOI: 10.1117/12.796100  0.683
2008 Barbour LW, Pensack RD, Hegadorn M, Arzhantsev S, Asbury JB. Excitation transport and charge separation in an organic photovoltaic material: Watching excitations diffuse to interfaces Journal of Physical Chemistry C. 112: 3926-3934. DOI: 10.1021/Jp0759628  0.72
2008 Asbury JB, Barbour LW, Pensack RD. Watching excitations diffuse and charges recombine at interfaces in organic photovoltaic materials Acs National Meeting Book of Abstracts.  0.656
2007 Barbour LW, Hegadorn M, Asbury JB. Watching electrons move in real time: ultrafast infrared spectroscopy of a polymer blend photovoltaic material. Journal of the American Chemical Society. 129: 15884-94. PMID 18044890 DOI: 10.1021/Ja074657X  0.465
2006 Barbour LW, Hegadorn M, Asbury JB. Microscopic inhomogeneity and ultrafast orientational motion in an organic photovoltaic bulk heterojunction thin film studied with 2D IR vibrational spectroscopy. The Journal of Physical Chemistry. B. 110: 24281-6. PMID 17134176 DOI: 10.1021/Jp065639P  0.468
2006 Zheng J, Kwak K, Chen X, Asbury JB, Fayer MD. Formation and dissociation of intra-intermolecular hydrogen-bonded solute-solvent complexes: chemical exchange two-dimensional infrared vibrational echo spectroscopy. Journal of the American Chemical Society. 128: 2977-87. PMID 16506778 DOI: 10.1021/Ja0570584  0.654
2005 Zheng J, Kwak K, Steinel T, Asbury J, Chen X, Xie J, Fayer MD. Accidental vibrational degeneracy in vibrational excited states observed with ultrafast two-dimensional IR vibrational echo spectroscopy. The Journal of Chemical Physics. 123: 164301. PMID 16268691 DOI: 10.1063/1.2071967  0.662
2005 Zheng J, Kwak K, Asbury J, Chen X, Piletic IR, Fayer MD. Ultrafast dynamics of solute-solvent complexation observed at thermal equilibrium in real time. Science (New York, N.Y.). 309: 1338-43. PMID 16081697 DOI: 10.1126/Science.1116213  0.782
2005 Asbury JB, Steinel T, Fayer MD. Vibrational echo correlation spectroscopy a new probe of hydrogen bond dynamics in water and methanol Femtosecond Laser Spectroscopy. 167-196. DOI: 10.1007/0-387-23294-X_7  0.501
2004 Asbury JB, Steinel T, Fayer MD. Vibrational echo correlation spectroscopy probes of hydrogen bond dynamics in water and methanol. Journal of Luminescence. 107: 271-286. PMID 19180255 DOI: 10.1016/J.Jlumin.2003.12.035  0.569
2004 Steinel T, Asbury JB, Zheng J, Fayer MD. Watching Hydrogen Bonds Break: A Transient Absorption Study of Water. The Journal of Physical Chemistry. A. 108: 10957-10964. PMID 19096727 DOI: 10.1021/Jp046711R  0.663
2004 Asbury JB, Steinel T, Kwak K, Corcelli SA, Lawrence CP, Skinner JL, Fayer MD. Dynamics of water probed with vibrational echo correlation spectroscopy. The Journal of Chemical Physics. 121: 12431-46. PMID 15606264 DOI: 10.1063/1.1818107  0.558
2004 Corcelli SA, Lawrence CP, Asbury JB, Steinel T, Fayer MD, Skinner JL. Spectral diffusion in a fluctuating charge model of water. The Journal of Chemical Physics. 121: 8897-900. PMID 15527354 DOI: 10.1063/1.1803532  0.563
2004 Asbury JB, Steinel T, Fayer MD. Hydrogen bond networks: Structure and evolution after hydrogen bond breaking Journal of Physical Chemistry B. 108: 6544-6554. DOI: 10.1021/Jp036600C  0.57
2004 Asbury JB, Steinel T, Stromberg C, Corcelli SA, Lawrence CP, Skinner JL, Fayer MD. Water dynamics: Vibrational echo correlation spectroscopy and comparison to molecular dynamics simulations Journal of Physical Chemistry A. 108: 1107-1119. DOI: 10.1021/Jp036266K  0.808
2004 Steinel T, Asbury JB, Corcelli SA, Lawrence CP, Skinner JL, Fayer MD. Water dynamics: Dependence on local structure probed with vibrational echo correlation spectroscopy Chemical Physics Letters. 386: 295-300. DOI: 10.1016/J.Cplett.2004.01.042  0.539
2003 Asbury JB, Steinel T, Stromberg C, Gaffney KJ, Piletic IR, Goun A, Fayer MD. Hydrogen bond dynamics probed with ultrafast infrared heterodyne-detected multidimensional vibrational stimulated echoes. Physical Review Letters. 91: 237402. PMID 14683215 DOI: 10.1103/Physrevlett.91.237402  0.776
2003 Asbury JB, Steinel T, Stromberg C, Gaffney KJ, Piletic IR, Fayer MD. Hydrogen bond breaking probed with multidimensional stimulated vibrational echo correlation spectroscopy Journal of Chemical Physics. 119: 12981-12997. DOI: 10.1063/1.1627762  0.791
2003 Asbury JB, Steinel T, Stromberg C, Gaffney KJ, Piletic IR, Goun A, Fayer MD. Ultrafast heterodyne detected infrared multidimensional vibrational stimulated echo studies of hydrogen bond dynamics Chemical Physics Letters. 374: 362-371. DOI: 10.1016/S0009-2614(03)00643-2  0.787
2003 Asbury JB, Steinel T, Fayer MD. Using ultrafast infrared multidimensional correlation spectroscopy to aid in vibrational spectral peak assignments Chemical Physics Letters. 381: 139-146. DOI: 10.1016/J.Cplett.2003.09.113  0.549
2003 Ai X, Anderson NA, Asbury JB, Hao E, Lian T. Ultrafast electron injection from adsorbates to semiconductor nanoparticles Proceedings of Spie - the International Society For Optical Engineering. 5223: 147-158.  0.451
2003 Asbury JB, Anderson NA, Hao E, Ai X, Lian T. Parameters affecting electron injection dynamics from ruthenium dyes to titanium dioxide nanocrystalline thin film Journal of Physical Chemistry B. 107: 7376-7386.  0.496
2002 Asbury JB, Wang Y, Lian T. Time-dependent vibration stokes shift during solvation: Experiment and theory Bulletin of the Chemical Society of Japan. 75: 973-983. DOI: 10.1246/Bcsj.75.973  0.547
2002 Hao E, Anderson NA, Asbury JB, Lian T. Effect of trap states on interfacial electron transfer between molecular absorbates and semiconductor nanoparticles Journal of Physical Chemistry B. 106: 10191-10198. DOI: 10.1021/Jp021226M  0.53
2001 Asbury JB, Wang YQ, Hao E, Ghosh HN, Lian T. Evidences of hot excited state electron injection from sensitizer molecules to TiO2 nanocrystalline thin films Research On Chemical Intermediates. 27: 393-406. DOI: 10.1163/156856701104202255  0.693
2001 Asbury JB, Hao E, Wang Y, Ghosh HN, Lian T. Ultrafast electron transfer dynamics from molecular adsorbates to semiconductor nanocrystalline thin films Journal of Physical Chemistry B. 105: 4545-4557. DOI: 10.1021/Jp003485M  0.593
2000 Wang Y, Asbury JB, Lian T. Ultrafast excited-state dynamics of Re(CO)3Cl(dcbpy) in solution and on nanocrystalline TiO2 and ZrO2 thin films Journal of Physical Chemistry A. 104: 4291-4299. DOI: 10.1021/Jp9936648  0.619
2000 Asbury JB, Hang K, Yeston JS, Cordaro JG, Bergman RG, Lian T. Direct observation of a picosecond alkane C-H bond activation reaction at iridium [4] Journal of the American Chemical Society. 122: 12870-12871. DOI: 10.1021/Ja0028065  0.446
2000 Anderson NA, Hang K, Asbury JB, Lian T. Ultrafast mid-IR detection of the direct precursor to the presolvated electron following electron ejection from ferrocyanide Chemical Physics Letters. 329: 386-392. DOI: 10.1016/S0009-2614(00)01046-0  0.547
1999 Asbury JB, Ellingson RJ, Ghosh HN, Ferrere S, Nozik AJ, Lian T. Femtosecond IR Study of Excited-State Relaxation and Electron-Injection Dynamics of Ru(dcbpy)2(NCS)2in Solution and on Nanocrystalline TiO2and Al2O3Thin Films The Journal of Physical Chemistry B. 103: 3110-3119. DOI: 10.1021/Jp983915X  0.688
1999 Asbury JB, Ellingson RJ, Ghosh HN, Ferrere S, Nozik AJ, Lian T. Femtosecond IR study of excited-state relaxation and electron-injection dynamics of Ru(dcbpy)2(NCS)2 in solution and on nanocrystalline TiO2 and Al2O3 thin films Journal of Physical Chemistry B. 103: 3110-3119.  0.304
1999 Ellingson RJ, Asbury JB, Ferrere S, Ghosh HN, Sprague JR, Lian T, Nozik AJ. Sub-picosecond injection of electrons from excited [Ru(2,2′-bipy-4,4′-dicarboxy)2(SCN)2] into TiO2 using transient mid-infrared spectroscopy Zeitschrift Fur Physikalische Chemie. 212: 77-84.  0.558
1998 Asbury JB, Ghosh HN, Yeston JS, Bergman RG, Lian T. Sub-Picosecond IR Study of the Reactive Intermediate in an Alkane C−H Bond Activation Reaction by CpRh(CO)2 Organometallics. 17: 3417-3419. DOI: 10.1021/Om980194F  0.622
1998 Ghosh HN, Asbury JB, Lian T. Direct observation of ultrafast electron injection from coumarin 343 to TiO2 nanoparticles by femtosecond infrared spectroscopy Journal of Physical Chemistry B. 102: 6482-6486.  0.514
1998 Ghosh HN, Asbury JB, Weng Y, Lian T. Interfacial electron transfer between Fe(II)(CN)6 4-and TiO2 nanoparticles: Direct electron injection and nonexponential recombination Journal of Physical Chemistry B. 102: 10208-10215.  0.496
1998 Asbury JB, Ghosh HN, Ellingson RJ, Ferrere S, Nozik AJ, Lian T. Femtosecond IR study of Ru(II)(SCN)2(dcbpy)2 sensitized nanocrystalline TiO2 thin films: Ultrafast electron injection and relaxation dynamics Springer Series in Chemical Physics. 63: 639-641.  0.541
1998 Ellingson RJ, Asbury JB, Ferrere S, Ghosh HN, Sprague JR, Lian T, Nozik AJ. Dynamics of electron injection in nanocrystalline titanium dioxide films sensitized with [Ru(4,4′-dicarboxy-2,2′-bipyridine)2(NCS)2] by infrared transient absorption Journal of Physical Chemistry B. 102: 6455-6458.  0.556
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